Visualization of superparamagnetic dynamics in magnetic topological insulators


  Ella O. Lachman [1]  ,  Andrea. F. Young [2]  ,  Anthony Richardella [3]  ,  Jo Cuppens [1]  ,  Naren HR [1]  ,  Yonathan Anahory [1]  ,  Alexander Y. Meltzer [1]  ,  Abhinav Kandala [3]  ,  Susan Kempinger [3]  ,  Yuri Myasoedov [1]  ,  Martin E. Huber [4]  ,  Nitin Samarth [3]  ,  Eli Zeldov [1]  
[1] Department of Condensed Matter Physics, Weizmann Institute of Science Rehovot 76100, Israel
[2] Physics Department, University of California Santa Barbara 93106-9530, USA
[3] Department of Physics, The Pennsylvania State University University Park, Pennsylvania 16802, USA
[4] Department of Physics, University of Colorado Denver Denver, Colorado 80217, USA

Magnetically doped topological insulators have recently been shown to host a quantum anomalous Hall state at low temperatures.  In the theoretical literature, the magnetic structure that underlies this topological state has been assumed to consist of long range magnetic order, with the polarization transition mediated by domain walls hosting topological edge states.  Transport and global magnetometry measurements are consistent with this idea, suggesting that the quantized resistance emerges from the breaking of time reversal symmetry in the form of large ferromagnetic domains. 

Using scanning nanoSQUID magnetic imaging on a Cr-doped (Bi,Sb)2Te3 thin film, we reveal that the magnetic structure is in fact a superparamagnetic state formed by weakly interacting magnetic domains. These domains have a characteristic size of a few tens of nanometers, and undergo random reversals which drive the electronic state from one Hall plateau to the other.
The superparamagnetic state is metastable, with very small energy barriers to relaxation. We observe magnetic relaxation on laboratory time scales even at 300 mK, evident also in transport measurements.  Unexpectedly, magnetic relaxation can also be induced by varying the back gate voltage, and we propose a mechanism for the influence of the electronic phase on the magnetic relaxation.  We speculate that the dynamic nature of magnetic disorder in quantum anomalous Hall systems may be at least partially responsible for the observed fragility of the quantum anomalous hall state at elevated temperatures.